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Bhartia, P. K.

Publications and source records attributed to Bhartia, P. K..

At least 55 records · Page 3

A Comparison of TOMS Version 8 Total Column Ozone Data with Data from Groundstations

The Nimbus-7 and Earth Probe Total Ozone Mapping Spectrometer (TOMS) data have been reprocessed with a new retrieval algorithm, (Version 8) and an updated calibration procedure. These data have been systematically compared to total ozone data from Brewer and Dobson spectrophotometers for 73 individual ground stations. The comparisons were made as a function of latitude, solar zenith angle, reflectivity and total ozone. Results show that the accuracy of the TOMS retrieval'is much improved when aerosols are present in the atmosphere, when snow/ice and sea glint are present, and when ozone in the northern hemisphere is extremely low. TOMS overpass data are derived from the single TOMS best match measurement, almost always located within one degree of the ground station and usually made within an hour of local noon. The version 8 Earth Probe TOMS ozone values have decreased by an average of about 1% due to a much better understanding of the calibration of the instrument. The remaining differences between TOMS and ground stations suggest that there are still small errors in the TOMS retrievals. But if TOMS is used as a transfer standard to compare ground stations, the large station-to-station differences suggest the possibility of significant instrument errors at some ground stations.

Labow, G. J.↗

Contribution of TOMS to Earth Science- An Overview

The TOMS instrument was launched on the Nimbus-7 satellite in Oct 1978 with the goal of understanding the meteorological influences on the ozone column. The nominal lifetime of the instrument was 1 year. However, in response to the concern over possible man-made influences on the ozone layer NASA continued to nurse the instrument for 13.5 years and launched a major program to produce accurate trend quality dataset of ozone. Despite severe optical degradation and other significant anomalies that developed in the instrument over its lifetime, the effort turned out to be a tremendous success. In 1984, TOMS took center stage as the primary provider of Antarctic ozone hole maps to the world community; it continues to play that role until today. An unexpected benefit of the close attention paid to improving the TOMS data quality was that several atmospheric constituents that interfere with ozone measurement were also identified and meticulously converted into long-term datasets of their own. These constituents include clouds, volcanic S02, aerosols, and ocean phytoplankton. In addition, the high quality of the basic datasets made it possible to produce global maps of surface UV and tropospheric ozone. In most cases there are no other sources of these data sets. Advanced UV instruments currently under development in the US and Europe will continue to exploit the TOMS-developed techniques for several decades.

Bhartia, P. K.↗

Improving Total Column Ozone Retrievals by Using Cloud Pressures Derived from Raman Scattering in the UV

The higher spectral resolution, coverage, and sampling of the Aura satellite ozone monitoring instrument (OMI), as compared with the total ozone mapping spectrometer (TOMS) should allow for improved ozone retrievals, including estimates of tropospheric ozone. By default, the TOMS-like OMI total column ozone algorithm uses climatological cloud-top pressures based on infrared (IR) measurements to estimate the column ozone below the clouds. Alternatively, cloud pressure can be retrieved using atmospheric rotational Raman scattering with OMI. The retrieved cloud pressures should be more consistent with assumptions made in the total ozone algorithm. Here, we use data from the global ozone monitoring experiment (GOME) to estimate total ozone using both the IR-climatological and retrieved cloud pressures. The exceed approximately 15 DU. Use of the UV cloud pressure retrievals leads to a smoother distribution of ozone along a satellite track by reducing small spatial irregularities presumably caused by errors in the climatological cloud pressures.

Vasilkov, A.↗

The EOS Aura Mission

The Earth Observing System (EOS) Aura satellite is scheduled to launch in the second quarter of 2004. The Aura mission is designed to attack three science questions: (1) Is the ozone layer recovering as expected? (2) What are the sources and processes that control tropospheric pollutants? (3) What is the quantitative impact of constituents on climate change? Aura will answer these questions by globally measuring a comprehensive set of trace gases and aerosols at high vertical and horizontal resolution. Fig. 1 shows the Aura spacecraft and its four instruments.

Schoebert, Mark R.↗

Aerosol Absorption Effects in the TOMS UV Algorithm

The availability of global long-term estimates of surface UV radiation is very important, not only for preventive medicine considerations, but also as an important tool to monitor the effects of the stratospheric ozone recovery expected to occur in the next few decades as a result of the decline of the stratospheric chlorine levels. In addition to the modulating effects of ozone and clouds, aerosols also affect the levels of UV-A and W-B radiation reaching the surface. Oscillations in surface W associated with the effects of aerosol absorption may be comparable in magnitude to variations associated with the stratospheric ozone recovery. Thus, the accurate calculation of surface W radiation requires that both the scattering and absorption effects of tropospheric aerosols be taken into account. Although absorption effects of dust and elevated carbonaceous aerosols are already accounted for using Aerosol Index technique, this approach does not work for urban/industrial aerosols in the planetary boundary layer. The use of the new TOMS long-term global data record on UV aerosol absorption optical depth, can improve the accuracy of TOMS spectral UV products, by properly including the spectral attenuation effects of carbonaceous, urban/industrial and mineral aerosols. The TOMS data set on aerosol properties will be discussed, and results of its use in the TOMS surface W algorithm will be presented.

Torres, O.↗

Retrieval of Total Ozone Amounts from Zenith-Sky Intensities in the Ultraviolet Region

A new method to determine the total ozone column from zenith-sky intensities in the ultraviolet region has been developed for the Shuttle Solar Backscatter Ultraviolet Spectrometer (SSBUV) operating at the NASA Goddard Space Flight Center. The total ozone column amounts are derived by comparing the ratio of measured intensities from three wavelengths with the equivalent ratios calculated by a radiative transfer model. The differences between the retrieved ozone column amounts and the collocated Brewer double monochromator are within 2% for the measurement period beginning in April 2001. The methodology, as well as the influences of the ozone profiles, aerosols, surface albedo, and the solar zenith angle on the retrieved total ozone amounts will be presented.

Bojkov, B. R.↗

Comparison of TOMS, SBW & SBUV/2 Version 8 Total Column Ozone Data with Data from Groundstations

The Nimbus-7 and Earth Probe Total Ozone Mapping Spectrometer (TOMS) data as well as SBUV and SBUV/2 data have been reprocessed with a new retrieval algorithm (Version 8) and an updated calibration procedure. An overview will be presented systematically comparing ozone values to an ensemble of Brewer and Dobson spectrophotometers. The comparisons were made as a function of latitude, solar zenith angle, reflectivity and total ozone. Results show that the accuracy of the TOMS retrieval has been improved when aerosols are present in the atmosphere, when snow/ice and sea glint are present, and when ozone in the northern hemisphere is extremely low. TOMS overpass data are derived from the single TOMS best match measurement, almost always located within one degree of the ground station and usually made within an hour of local noon. The Version 8 Earth Probe TOMS ozone values have decreased by an average of about 1% due to a much better understanding of the calibration of the instrument. N-7 SBUV as well as the series of NOAA SBUV/2 column ozone values have also been processed with the Version 8 algorithm and have been compared to values from an ensemble of groundstations. Results show that the SBW column ozone values agree well with the groundstations and the datasets are useful for trend studies.

Labow, G. J.↗

Validation of SCIAMACHY and TOMS UV Radiances Using Ground and Space Observations

Verification of a stratospheric ozone recovery remains a high priority for environmental research and policy definition. Models predict an ozone recovery at a much lower rate than the measured depletion rate observed to date. Therefore improved precision of the satellite and ground ozone observing systems are required over the long term to verify its recovery. We show that validation of satellite radiances from space and from the ground can be a very effective means for correcting long term drifts of backscatter type satellite measurements and can be used to cross calibrate all B W instruments in orbit (TOMS, SBW/2, GOME, SCIAMACHY, OM, GOME-2, OMPS). This method bypasses the retrieval algorithms used for both satellite and ground based measurements that are normally used to validate and correct the satellite data. Radiance comparisons employ forward models and are inherently more accurate than inverse (retrieval) algorithms. This approach however requires well calibrated instruments and an accurate radiative transfer model that accounts for aerosols. TOMS and SCIAMACHY calibrations are checked to demonstrate this method and to demonstrate applicability for long term trends.

Hilsenrath, E.↗

The Antarctic Ozone Hole: Initial Results from Aura / OMI Compared with TOMS

A series of TOMS instruments (on November 7 , Meteor 3, and Earth Probe) has been monitoring the annual development of the Antarctic ozone hole since the 1980s. The ozone mapping instrument on Aura, OMI, is expected to take over this record of observation from the aging Earth Probe TOMS instrument. The area of the ozone hole can be taken as a sensitive indicator of the magnitude of ozone destruction each year. The timing of initial formation of the ozone hole and its duration are sensitive to the atmospheric dynamics of the southern polar regions. The entire TOMS data record (1978 - 2004) has recently been reprocessed with the new version 8 algorithm, which includes a revised calibration. The effect has been to slightly increase ozone hole area over earlier estimates, but only by 23%. OMI (ozone monitoring instrument) on Aura is a hyperspectral imaging instrument that operates in a pushbroom mode to measure solar backscattered radiation in the ultraviolet and visible. OMI has higher spatial resolution than TOMS - 14 x 24 km versus 38 km x 38 km from TOMS. OMI has now begin mapping total column ozone on a global basis in a measurement similar to TOMS. The ozone hole measurements for 2003 are compared with those from Earth Probe TOMS.

McPeters, R.↗

Validation of SCIAMACHY Radiances and Ozone Products Using Ground and Space Observations

Validation of SCIAMACHY data products are is key element for the detecting a stratospheric ozone recovery, which is a high priority for environmental research and environmental policy. Models predict an ozone recovery at a much lower rate than the measured depletion rate observed to date. Therefore improved precision of the satellite and ground ozone observing systems are required over the long term to verify its recovery. We show that validation of satellite radiances from space and from the ground can be an effective means for correcting long term drifts of backscatter type satellite measurements such as SCIAMACHY and can be used to cross calibrate all BUV instruments in orbit (TOMS, SBUV/2, GOME, OMI, GOME-2, OMPS). This method bypasses the retrieval algorithms used for both satellite and ground based measurements that are normally used to validate and correct the satellite data. This approach however requires well calibrated instruments and an accurate radiative transfer model that accounts for aerosols. In addition to comparing radiances, validation of SCIAMACHY ozone products will conducted by comparing total and profile ozone with TOMS and SBUV/2.

Hilsenrath, E.↗

Ozone Profiles and Tropospheric Ozone from Global Ozone Monitoring Experiment

Ozone profiles are derived from backscattered radiances in the ultraviolet spectra (290-340 nm) measured by the nadir-viewing Global Ozone Monitoring Experiment using optimal estimation. Tropospheric O3 is directly retrieved with the tropopause as one of the retrieval levels. To optimize the retrieval and improve the fitting precision needed for tropospheric O3, we perform extensive wavelength and radiometric calibrations and improve forward model inputs. Retrieved O3 profiles and tropospheric O3 agree well with coincident ozonesonde measurements, and the integrated total O3 agrees very well with Earth Probe TOMS and Dobson/Brewer total O3. The global distribution of tropospheric O3 clearly shows the influences of biomass burning, convection, and air pollution, and is generally consistent with our current understanding.

Liu, X.↗

Retrieval Studies with LIDORT

This short program of LIDORT-based research in atmospheric trace gas retrieval was conducted over the 1 year period 01 July 2002 to 30 June 2003. After consultation with the NASA reporting officer, the first of the two original proposal activities (development of a direct-fitting total O3 column retrieval algorithm with operational capability for GOME data) was replaced by other tasks. The three activities addressed were: (1) Sensitivity studies for column and profile retrieval of NO2 distributions from a new generation of multi-axis ground-based spectrometers; (2) use of the LIDORT-RRS model to determine the effect of inelastic rotational Raman scattering at SBUV wavelengths; (3) an examination of ozone profile weighting functions in the presence of optically thick tropospheric clouds.

Bhartia, P. K.↗

Using Cloud Top Pressures Derived from Raman Scattering in the UV for the OMI Total Column Ozone Retrievals

The OMI cloud pressure product is necessary for accounting for cloud effects on the mission- critical total ozone product. One of the OM1 cloud pressure algorithms uses UV measurements to derive cloud pressures from the high frequency structure of top- of-atmosphere reflectance caused by rotational Raman scattering (RRS) in the atmosphere. RRS results in filling-in of Fraunhofer lines in the backscatter UV spectra (also known as the Ring effect). The magnitude of filling-in of the Fraunhofer lines is roughly proportional to the average number of solar photon scatterings in the atmosphere above the clouds. This property of RRS is used to deduce an effective cloud pressure. The cloud pressure algorithm retrieves the cloud pressure and cloud fraction using a concept of the Mixed Lambert Equivalent Reflectivity (MLER) also used for the TOMS-V8 OM1 total column ozone algorithm. Currently, this OMI total column ozone algorithm utilizes information about cloud top pressures from a climatology based on IR measurements. The IR-derived cloud top pressure is known to be lower than UV-derived cloud top pressure because UV radiation penetrates clouds deeper than IR radiation. That is why the UV-derived cloud pressure may be more consistent withthe total ozone algorithm. We estimate total column ozone differences caused by replacing the cloud pressure climatology with cloud pressures retrieved from GOME data same as used for retrieval of ozone.

Joiner, J.↗

Properties of Backscattered Ultraviolet Reflectances in Cloudy Atmosphere

We use a Plane-Parallel Cloud (PPC) model to illustrate how Mie scattering from cloud particles interacts with Rayleigh scattering in the atmosphere and produces a complex wavelength dependence in the top-of-the-atmosphere (TOA) reflectances measured by satellite instruments that operate in the ultraviolet (UV) part of the spectrum. Comparisons of the PPC model-derived spectral dependence of reflectances with the Total Ozone Mapping Spectrometer (TOMS) measurements show surprisingly good agreement over a wide range of observational conditions. The PPC model results also are compared with the results of two other cloud models: Lambert Equivalent Reflectivity (LER) and Modified Lambert Equivalent Reflectivity (MLER) that have been used to analyze satellite data in the UV. These models assume that clouds are opaque Lambertian reflectors rather than Mie scattering particles. Although one of these models (MLER) agrees reasonably well with the data, the results from this model appear somewhat unphysical and may not be suitable for interpreting satellite data if one desires high accuracy. We also use the PPC model to illustrate how clouds can perturb tropospheric O3 absorption in complex ways that cannot be explained by models that treat them as reflecting surfaces rather than as volume scatterers.

Ahmad, Z.↗

The Updated Umkehr Ozone Retrieval Algorithm and its Validation against Satellite Data

Improvements to the Umkehr ozone profile retrieval algorithm have been developed and are now being evaluated. The updated algorithm is able to simulate observations more accurately and provides data output that is easier to analyze. Among the new diagnostic capabilities that the updated algorithm provides is the averaging kernel (AK) method. The AK approach allows studying how the algorithm responds when a small perturbation is made in a particular layer of the atmosphere [Rodgers 1976, 1990]. We will use the AK method to define precisely what Umkehr should measure given a set of profiles measured by other platforms. This method allows us to compare trends and offsets in data more accurately than it has been done in the past. The updated Umkehr retrievals will be validated against SAGE II ozone profiles as well as SSBUV ozone profile data. We will discuss possible reasons for offset between data and differences in derived ozone profile trends. Considerable variability of the ozone profile within the 10-degree latitude envelope creates noise in the SAGE matching dataset and makes comparisons difficult. To eliminate this problem, the SAGE and Umkehr data had been previously de-seasonalized by subtracting the latitude/season dependent ozone climatology. However, the remaining noise in the ozone residuals was still considerably high for trend analysis and was attributed to longitude variability of SAGE sampling. The new ozone climatology (Labow, NASA) that has longitude dependent ozone variability will be used to minimize contribution of sampling noise in comparisons of satellite and ground station. The comparison of zenith-sky radiances (Umkehr N-value measurements) synthesized for a given set of SAGE profiles will be used to determine whether SAGE-derived N-values agree with the Umkehr-measured N-values. The instrumental effects will be discussed. Both the Umkehr data and SAGE II measurements will be analyzed for their information about ozone variability and loss and recovery rates at the mid- and upper (40 km) levels. The updated long-term Umkehr dataset can be used to provide high quality information for identifying signs of ozone recovery. The long Umkehr historical record can provide additional information for separating the dynamic and chemical mechanisms of depletion, and can help the community better understand climate change effects.

Petropavlovskikh, I.↗

New Total Ozone Algorithm for Application to the Total Ozone Mapping Spectrometer

The Total Ozone Mapping Spectrometer (TOMS) series comprises four instruments providing a total of 25 years of daily global stratospheric ozone data over the sunlit portion of the Earth. A new retrieval algorithm has been developed for TOMS, designated Version 8. The algorithm is based on differential absorption across a pair of wavelength channels chosen close together to minimize the impact of wavelength dependent forward modeling errors. Version 8 enhancements include correction for the presence of tropospheric aerosols and sun glint from water surfaces, a better treatment of variability due to tropospheric ozone and temperature dependence, and an improved forward model, particularly in regions of persistent snow and ice. Among other things, the Version 8 enhancements have reduced latitudinal dependence seen previously in TOMS - Dobson comparisons, predominantly in the Southern Hemisphere's summer, when the tropospheric ozone, temperature, and snow/ice corrections are additive. The basic components of the algorithm and its impact on derived total ozone will be discussed.

Wellemeyer, C.↗

EOS-Aura's Ozone Monitoring Instrument (OMI): Validation Requirements

OMI is an advanced hyperspectral instrument that measures backscattered radiation in the UV and visible. It will be flown as part of the EOS Aura mission and provide data on atmospheric chemistry that is highly synergistic with other Aura instruments HIRDLS, MLS, and TES. OMI is designed to measure total ozone, aerosols, cloud information, and UV irradiances, continuing the TOMS series of global mapped products but with higher spatial resolution. In addition its hyperspectral capability enables measurements of trace gases such as SO2, NO2, HCHO, BrO, and OClO. A plan for validation of the various OM1 products is now being formulated. Validation of the total column and UVB products will rely heavily on existing networks of instruments, like NDSC. NASA and its European partners are planning aircraft missions for the validation of Aura instruments. New instruments and techniques (DOAS systems for example) will need to be developed, both ground and aircraft based. Lidar systems are needed for validation of the vertical distributions of ozone, aerosols, NO2 and possibly SO2. The validation emphasis will be on the retrieval of these products under polluted conditions. This is challenging because they often depend on the tropospheric profiles of the product in question, and because of large spatial variations in the troposphere. Most existing ground stations are located in, and equipped for, pristine environments. This is also true for almost all NDSC stations. OMI validation will need ground based sites in polluted environments and specially developed instruments, complementing the existing instrumentation.

Brinksma, E. J.↗

Total Ozone from the Ozone Monitoring System (OMI) using TOMS and DOAS Methods

The Ozone Monitoring Instrument (OMI) is the Dutch-Finnish contribution to NASA's EOS-Aura satellite scheduled for launch in January 2004. OMI is an imaging spectrometer that will measure the back-scattered Solar radiance in the wavelength range of 270 to 500 nm. The instrument provides near global coverage in one day with a spatial resolution of 13x24 square kilometers. OMI is a new instrument, with a heritage from TOMS, SBW, GOME, GOMOS and SCIAMACHY. OMI'S unique capabilities for measuring important trace gases and aerosols with a small footprint and daily global coverage, in conjunction with the other Aura instruments, will make a major contribution to our understanding of stratospheric and tropospheric chemistry and climate change. OMI will provide data continuity with the 23-year ozone record of TOMS. There are three ozone products planned for OMI: total column ozone, ozone profile and tropospheric column ozone. We are developing two different algorithms for total column ozone: one similar to the algorithm currently being used to process the TOMS data, and the other an improved version of the differential optical absorption spectroscopy (DOAS) method, which has been applied to GOME and SCIAMACHY data. The main reasons for starting with two algorithms for total ozone have to do with heritage and past experience; our long-term goal is to combine the two to develop a more accurate and reliable total ozone product for OMI. We will compare the performance of these two algorithms by applying both of them to the GOME data. We will examine where and how the results differ, and use the extensive TOMS-Dobson comparison studies to assess the performance of the DOAS algorithm.

Veefkind, J. P.↗