Aerosol Humidification Observed by the Airborne High Spectral Resolution Lidar-2
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Engineering topics
Publications and source records attributed to Allison Collow.
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Atmospheric rivers (ARs) are long, narrow synoptic scale features that act as moisture transport vehicles by moving water vapor poleward. They are typically found in storm tracks and often have profound implications for regional hydroclimate. For high latitude locales such as Antarctica and the Arctic, ARs are fewer in number but often have an outsized impact by either producing significant snow accumulation events, or, depending on their thermal characteristics, initiating melt events on ice sheets, ice shelves, and sea ice. In this study, we apply both reanalysis and climate model data to evaluate high latitude ARs for both the Arctic and Antarctic in the context of teleconnections and modes of variability. Specifically, we fold in both MERRA-2 and ERA5 reanalysis as well as historical and climate change simulations from the CESM2 (Community Earth System Model, Version 2) and E3SMv2 (Energy Exascale Earth System Model, v2) with multiple ensemble members to better understand natural variability versus climate change signals. An overview of AR climatology and impacts will be presented, including a baseline uncertainty quantification analysis using data from ARTMIP (the Atmospheric River Tracking Method Intercomparison Project). AR impacts during specific modes of variability will be characterized by diagnosing precipitation and boundary layer temperature associated with Ars influencing the cryosphere. Modes of variability investigated include the SAM (Southern Annular Mode), PDO (Pacific Decadal Oscillation), PSA2 (Pacific South American Mode 2), the IOD (Indian Ocean Dipole), and the AO (Arctic Oscillation).
The Goddard Chemistry Aerosol Radiation and Transport (GOCART) model, which controls the sources sinks and chemistry within the Goddard Earth Observing System, recently underwent a major refactoring and update to the representation of physical processes. The code refactoring increases flexibility such multiple instances of an aerosol species can be run and interact with radiation and cloud microphysics, in addition to the output of multiple wavelength aerosol optical properties in support of data assimilation. From a science perspective, a new radiatively active tracer, brown carbon, was added to distinguish smoke from other sources of organic aerosol thereby improving optical properties entering the radiative calculations. A four-year benchmark simulation was evaluated using in situ and space borne measurements to develop a baseline and prioritize future development. A comparison of simulated aerosol optical depth between GOCART-2G and MODIS retrievals indicates the model captures the overall spatial pattern and seasonal cycle of aerosol optical depth but overestimates aerosol extinction over dusty regions and underestimates aerosol extinction over northern hemisphere boreal forests, requiring further tuning of emissions. This MODIS-based analysis is corroborated by comparisons to MISR and selected AERONET stations. Despite the underestimate of aerosol optical depth in biomass burning regions in GEOS, there is an overestimate in the surface mass of organic carbon in the United States, especially during the summer months.
In the first week of May 2023, boreal Canada began an early start to the biomass burning season when fires erupted across Alberta and western Saskatchewan. Smoke entered the troposphere and spread across the United States as biomass burning emissions in Canada quadrupled the prior maximum since the onset of the MODIS satellite record. Adding to the already existing smoke, wildfires ignited in Quebec on June 2, 2023, producing a heavy plume of aerosol over the northeastern part of the continent. Meteorological factors, including an area of low pressure situated, nearly stationary, over Maine, transported the smoke into a densely populated corridor containing the cities of Washington, DC, Baltimore, Philadelphia, and New York City. Air quality alerts became widespread as near-surface levels of fine particulate matter (PM2.5) exceeded harmful levels due the low altitude of the smoke plume. Forecasting the smoke transport and impacts of such events requires a complex combination of observed initial conditions for meteorology and aerosols, knowledge of the emissions from wildfires, and a state-of-the-art Earth System model that couples these components together. Using a case-study perspective with the Goddard Earth Observing System (GEOS), challenges associated with near real time forecasting of the smoke plume are presented. Analyzed and forecasted aerosol optical depth will be evaluated using available satellite and AERONET observations, while surface aerosol will be assessed relative to observations of PM2.5. Lacking real time estimates of biomass burning emissions for inputs to our forecast model, particular attention is given to the use of day-old biomass burning emissions throughout the forecast period covering the first ten days in June 2023, and the resulting reduction in forecast skill will be quantified.
In late December 2022 and the first half of January 2023, much of California experienced an unprecedented series of atmospheric rivers that produced heavy rains and near-record flooding. Previous work shows that a chain of dynamical events contributed to the extreme precipitation, including the development of a Rossby wave (as a result of forcing linked to the MJO) that emerged from the Indian Ocean in mid-December, and the subsequent development of a persistent positive Pacific North American (PNA) pattern that ultimately directed moisture onto the US West Coast starting in late December. Here, we use a stationary wave model (SWM) to further elucidate the dynamical and thermodynamical processes that drove the aforementioned chain of events. The results reveal the following: 1) The mid-December Rossby wave was likely induced by vorticity stretching and advection in the middle East linked indirectly to the MJO, 2) The initial development of the PNA in late December was triggered by transient and stretching sources of vorticity in the Pacific that were themselves induced by the aforementioned Rossby wave, and 3) The PNA was maintained through mid-January in part by diabatic heating west of Hawaii that was associated with anomalous precipitation influenced by the PNA circulation anomalies, thus representing a feedback on the PNA. One key finding from the SWM analysis is the limited direct role of tropical heating for inducing any of the dynamical mechanisms related to the California extreme event.
In the first week of May 2023, boreal Canada began an early start to the biomass burning season when fires erupted across Alberta and western Saskatchewan. Smoke entered the troposphere and spread across the United States as biomass burning emissions in Canada quadrupled the prior maximum since the onset of the MODIS satellite record. Adding to the already existing smoke, wildfires ignited in Quebec on June 2, 2023, producing a heavy plume of aerosol over the northeastern part of the continent. Meteorological factors, including an area of low pressure situated, nearly stationary, over Maine, transported the smoke into a densely populated corridor containing the cities of Washington, DC, Baltimore, Philadelphia, and New York City. Air quality alerts became widespread as near-surface levels of fine particulate matter (PM2.5) exceeded harmful levels due the low altitude of the smoke plume. Forecasting the smoke transport and impacts of such events requires a complex combination of observed initial conditions for meteorology and aerosols, knowledge of the emissions from wildfires, and a state-of-the-art Earth System model that couples these components together. Using a case-study perspective with the Goddard Earth Observing System (GEOS ), challenges associated with near real time forecasting of the smoke plume are presented. Analyzed and forecasted aerosol optical depth will be evaluated using available satellite and AERONET observations, while surface aerosol will be assessed relative to observations of PM2.5. Lacking real time estimates of biomass burning emissions for inputs to our forecast model, particular attention is given to the use of day-old biomass burning emissions throughout the forecast period covering the first ten days in June 2023, and the resulting reduction in forecast skill will be quantified.
The presence of fine particles in the atmosphere with a diameter of less than 2.5 µm, called particulate matter 2.5 (PM 2.5 ), poses a significant threat to human health as a criteria air pollutant. Fortunately, NASA's Goddard Earth Sciences Data and Information Services Center (GES DISC) provides easy access to several PM 2.5 concentration products. These datasets include the reanalysis of global hourly and monthly aerosol components including PM 2.5 data from the Modern-Era Retrospective analysis for Research and Applications, version 2 (MERRA-2), as well as 3-hourly real-time ensemble forecasts of PM 2.5 from the Hazardous Air Quality Ensemble System (HAQES). The HAQES products are developed by the George Mason University Air Quality Laboratory as part of NASA's Health Air Quality Applied Science Team (HAQAST). The GES DISC is actively collaborating with scientists in the HAQAST program to further expand air quality data collections. Two new datasets are currently being archived: one is the machine learning-based global hourly PM 2.5 derived from MERRA-2; the other is the localized data (NO 2 , O 3 , and PM 2.5 ) time series derived from NASA's GEOS Composition Forecasting (GEOS-CF) system. In this presentation, we will explore the spatial patterns and long-distance transport characteristics of elevated PM 2.5 during extreme pollution events, such as the June 2023 Canadian wildfires, which are still active at the time of writing; and severe spring dust storms in 2023 over Asia. To gain comprehensive insights, we will utilize various PM 2.5 data in conjunction with satellite-observed aerosol data from TROPOspheric Monitoring Instrument (TROPOMI) on Sentinel-5P. The primary focus of this presentation will be to demonstrate effective use of data tools and services to visualize and explore extreme air pollution phenomena. Additionally, we will provide guidance on how users can download specific data of interest, facilitating further analysis and research in this critical area.
Modeling of long-term trends of aerosols and their properties is important for constraining aerosol-climate forcing, and for characterizing changes in particulate matter pollution speciation and exposure. Here we study global and regional long-term trends in surface fine particulate matter (PM ) and aerosol optical properties for 60 years from 1958 to 2018, using simulations performed with the NASA Goddard Earth Observing System Chemistry Climate Model (GEOSCCM), and evaluate the model hindcast with observations for the last three decades. Comparing the modeled aerosols with a diverse set of observations helps interpret observed and simulated trends, and serves as a benchmark for future GEOSCCM developments and input datasets improvements. We first characterize modeled global and regional temporal changes in surface PM and its components, aerosol optical depth (AOD) and single scattering albedo (SSA) and we interpret their link with emissions drivers. We then compare modeled surface PM with ground-based observations from monitoring networks and with global reconstructed PM datasets from observations-model data fusion. Total AOD is compared with long-term satellite measurements from the Moderate Resolution Imaging Spectroradiometer (MODIS) and measurements from the ground-based Aerosol Robotic Network (AERONET). Additional aerosol optical properties, such as absorption and scattering coefficients, are evaluated with ground-based observations from the Global Atmosphere Watch (GAW) records.
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In late December 2022 and the first half of January 2023, much of California experienced an unprecedented series of atmospheric rivers that produced heavy rains and near-record flooding. Previous work shows that a chain of dynamical events contributed to the extreme precipitation, including the development of a Rossby wave (as a result of forcing linked to the MJO) that emerged from the Indian Ocean in mid-December, and the subsequent development of a persistent positive Pacific North American (PNA) pattern that ultimately directed moisture onto the US West Coast starting in late December. Here, we use a stationary wave model (SWM) to further elucidate the dynamical and thermodynamical processes that drove the aforementioned chain of events. The results reveal the following: 1) The mid-December Rossby wave was likely induced by vorticity stretching and advection in the middle East linked indirectly to the MJO, 2) The initial development of the PNA in late December was triggered by transient and stretching sources of vorticity in the Pacific that were themselves induced by the aforementioned Rossby wave, and 3) The PNA was maintained through mid-January in part by diabatic heating west of Hawaii that was associated with anomalous precipitation influenced by the PNA circulation anomalies, thus representing a feedback on the PNA. One key finding from the SWM analysis is the limited direct role of tropical heating for inducing any of the dynamical mechanisms related to the California extreme event.
Biomass burning aerosol impacts aspects of the atmosphere and Earth system through direct and semi-direct effects, as well as influencing air quality. Despite its importance, the representation of biomass burning aerosol is not always accurate in numerical weather prediction and climate models or reanalysis products. Using observations collected as part of the Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP2Ex) in August through October of 2019, aerosol concentration and optical properties are evaluated within the Goddard Earth Observing System (GEOS) and its underlying aerosol module, GOCART. In the operational configuration, GEOS assimilates aerosol optical depth observations at 550 nm from AERONET and MODIS to constrain aerosol fields. Particularly for biomass burning aerosol, without the assimilation of aerosol optical depth, aerosol extinction is underestimated compared to observations collected in the Philippines region during the CAMP2Ex campaign. The assimilation process adds excessive amounts of carbon to account for the underestimated extinction, resulting in positive biases in the mass of black and organic carbon, especially within the boundary layer, relative to in situ observations from the Langley Aerosol Research Group Experiment. Counteracting this, GEOS is deficient in sulfate and nitrate aerosol just above the boundary layer. Aerosol extinction within GEOS is a function of the mass of different aerosol species, the ambient relative humidity, the assumed spectral optical properties, and particle size distribution per species. The relationship between dry and ambient extinction in GEOS reveals that hygroscopic growth is too high within the model for biomass burning aerosol. An additional concern lies in the assumed particle size distribution for GEOS, which has a single mode radius that is too small for organic carbon. Variability in the observed particle size distribution for biomass burning aerosol within a single flight also illuminates the fact that a single assumed particle size distribution is not sufficient and that for a proper representation, a more advanced aerosol module within GEOS may be necessary.
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Over the past few years, NASA’s Global Modelling and Assimilation Office has been working on the configuration and production of three new reanalysis products, GEOS-IT, GiOcean, and MERRA-21C. GEOS-IT, or the Goddard Earth Observing System for Instrument Teams, is a 3D variational data assimilation system that runs in a near real time framework however retrospectively provides data back through 1998 to deliver a consistent view of the Earth-atmosphere system for the production of observational NASA products. Retrospective production for GEOS-IT is complete and the meteorology has since been used to produce the one way weakly coupled GiOcean reanalysis. Due to differences in the atmospheric model, particularly related to scavenging, aerosols are not identical in GEOS-IT and GiOcean. MERRA-21C, or the Modern Era Restrospective analysis for Research and Applications in the 21st century, is a hybrid 4D ensemble variational system at a finer horizontal resolution of 0.25 degrees. Although different in their intended use, and therefore configuration, these systems prominently feature coupling between meteorology and aerosols. The differences and similarities in the aerosol configuration between the three systems will be discussed, covering biomass burning and anthropogenic emissions as well as observations used for the assimilation of aerosol optical depth. A large emphasis will be placed on the version of the underlying aerosol module, GOCART, which underwent a complete refactoring and the addition of radiatively active brown carbon between GEOS-IT and MERRA-21C. Independent observations will be used to evaluate the performance of aerosols in both reanalyses, focusing on aerosol optical depth, surface particulate matter, and vertical profiles of aerosol backscatter.
During the initial planning of the Modern Era Retrospective-analysis for Research and Applications (MERRA), the project was envisioned to become a tool for applied sciences and decision makers, as well as weather and climate research. MERRA was the first reanalysis to provide data at 1 hourly frequencies. After discussions with wind energy users, 50m above the surface winds were included in the data collection to begin to represent the environment at the turbine height. MERRA-2 was the first reanalysis to include interactive and assimilated aerosols. From these, PM 1, 2.5 and 10 records have been computed and contribute to the climate and health sector. The US Center for Disease Control is accessing MERRA-2 data for comparison along with their health data. MERRA-2 Extreme Indices have been computed from the high frequency data (e.g. precipitation maxima, heat waves and fire weather). These have been used to characterize the changing extremes in the United States and around the globe as well as the weather associated with the extremes. The next-generation, MERRA-21C, includes increased resolution (25km) and continues to provide innovative Earth system data. For example, a boundary layer collection will provide constant height level data starting at 100m, continuing up to 4000m. This will provide detailed information about the boundary layer processes that greatly affect the biosphere. Chemical tracers for constituents are included in the system. The ensemble data assimilation is run with 32 members, and the variance for critical variables are stored. We will explore the use of this variance as one measure of uncertainty relevant for applied uses, which has not been included in any MERRA reanalysis. We will discuss use case scenarios developed to engage with the energy and financial sectors, to better understand their needs for climate data. Prospects for further downscaling of reanalyses will also be explored.
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Explore the source record for details and available documents.
Explore the source record for details and available documents.
Explore the source record for details and available documents.